Synthesis of Androprostamine A and Resormycin

Syntheses of androprostamine A (1), and resormycin (3), anti-prostate cancer peptidyl natural products produced by microorganisms, were completed. The characteristic enamide structures of these compounds were installed using the Horner-Wadsworth-Emmons reaction from the corresponding phosphonates in reasonable Z-selectivity.

Chemical & pharmaceutical bulletin. 2016 [Epub]

Hikaru Abe, Yohko Yamazaki, Chiharu Sakashita, Isao Momose, Takumi Watanabe, Masakatsu Shibasaki

Institute of Microbial Chemistry (BIKAKEN), Tokyo.